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The Structure Ligation Relationship (SLR) of free amino acids (AAs) under Pd‐catalysis were examined for the chemo‐ and regio‐selective indole C–H arylation reactions. While the majority of AAs were minor or ineffective, the L‐aspartic acid (L‐Asp) stands out promising to deliver high‐value C3–arylated indoles with excellent chemo‐ (C vs N) and regioselectivity (C3 vs C2) with high functional group tolerance. Thus, the protocol offers a cost‐effective and sustainable alternative of phosphine‐based ligands for the indole C3‐H arylation reactions. Preliminary mechanistic investigations suggested the simultaneous involvement of −NH2, α−CO2H, and β−CO2H functionalities of L‐Asp and found critical for its ligation efficiency. The developed catal.
FP Trading Desk (Canada) 05/29/2020 02:19
TOKYO — The yen rose against major currencies on Friday as caution ahead of U.S. President Donald Trump’s press conference on China’s treatment of Hong Kong triggered safe-haven inflows. The dollar drifted lower against the euro and the British pound but could quickly reverse course amid growing concern about tense relations between the world’s two […]
The Conversation 05/29/2020 02:15
Lucy Nicholson/Reuters. Australia’s latest greenhouse gas figures show national emissions fell slightly last year. This was by no means an economy-wide effort – solar and wind energy did most of the heavy lifting. Emissions fell 0.9% last year compared to 2018. The rapid deployment of solar and wind is slashing emissions in the electricity sector, offsetting increases from all other sectors combined. Read more:. Renewables (solar, wind and hydro) now comprise in the National Electricity Market. In 2023, renewables will likely pass black coal to become the largest electricity source. In an ideal world, all sectors of the economy – transport, agriculture, manufacturing and others – would pull in the same direction to cut emissions. But hearteni.

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